Relativistic heavy ion collisions provide a unique opportunity to probe the nuclear structure by taking an instantaneous snapshot of the col
Relativistic heavy ion collisions provide a unique opportunity to probe the nuclear structure by taking an instantaneous snapshot of the colliding nuclei and converting it into momentum anisotropies of final emitted hadrons. A long-standing puzzle of too large a ratio of the elliptical-to-triangular ($v_{2}$-to-$v_{3}$) anisotropies in ultracentral $^{208}$Pb+$^{208}$Pb collisions at the Large Hadron Collider(LHC) cannot be solved simply by hydrodynamic simulations with initial conditions containing the spherical or certain deformed shape of $^{208}$Pb. In this Letter, using the iEBE-VISHNU relativistic viscous hydrodynamic hybrid model simulations with the Trento initial condition, we show that a dynamic octupole deformation--a shape-breathing of $^{208}$Pb --could potentially solve the $v_{2}$-to-$v_{3}$ puzzle and simultaneously describe the $v_3\{4\}$ data measured in experiment. Our results highlight the unique capability of capturing transient collective properties of nuclei on yoctosecond ($10^{-24}$~s) timescales, unfeasible with low-energy nuclear reactions. Comment: 7 pages, 4 figures, version submitted for publication